| dc.creator |
Ramos, Ángel |
|
| dc.creator |
Tejeda, Guzmán |
|
| dc.creator |
Fernández Sánchez, José María |
|
| dc.creator |
Montero, Salvador |
|
| dc.date |
2008-02-07T14:32:38Z |
|
| dc.date |
2008-02-07T14:32:38Z |
|
| dc.date |
2005-11-09 |
|
| dc.date.accessioned |
2017-01-31T01:00:01Z |
|
| dc.date.available |
2017-01-31T01:00:01Z |
|
| dc.identifier |
Physical Review A 72, 053204 (2005) |
|
| dc.identifier |
1050-2947 |
|
| dc.identifier |
http://hdl.handle.net/10261/2891 |
|
| dc.identifier |
10.1103/PhysRevA.72.053204 |
|
| dc.identifier.uri |
http://dspace.mediu.edu.my:8181/xmlui/handle/10261/2891 |
|
| dc.description |
The condensation produced in supersonic expansions of CO2 is studied quantitatively combining Rayleigh and Raman scattering. The cluster number density nc and the mean cluster size <N> are obtained for five expansions with stagnation pressures P0=1-5 bars, and temperature T0=294 K, along axial and radial directions; nc and <N> are determined from the condensation onset up to a terminal size, verifying the empirical law <N>prop.P0^(2.23). A maximum growth rate d<N>/dt approx.8x10(8) s^(-1) is estimated for the 5-bar expansion. The Raman spectra show a coexistence of solid and liquidlike phases in the jet, with a progressive transition from the liquid to the solid fraction as the clusters increase their size. |
|
| dc.description |
Ministerio de Educación y Ciencia, Proyectos BFM2001-2276 y FIS2004-02576 |
|
| dc.description |
Peer reviewed |
|
| dc.format |
498061 bytes |
|
| dc.format |
application/pdf |
|
| dc.language |
eng |
|
| dc.publisher |
American Physical Society |
|
| dc.relation |
http://dx.doi.org/10.1103/PhysRevA.72.053204 |
|
| dc.rights |
openAccess |
|
| dc.subject |
Supersonic expansion |
|
| dc.subject |
Molecular clusters |
|
| dc.subject |
Raman spectroscopy |
|
| dc.subject |
Rayleigh scattering |
|
| dc.subject |
Cluster size distribution |
|
| dc.title |
Quantitative study of cluster growth in free-jet expansions of CO2 by Rayleigh and Raman scattering |
|
| dc.type |
Artículo |
|